Background and Purpose: Bark thickness and its share in the volume of roundwood are the most important characteristics of the bark, particularly in the process of timber harvesting, and during scaling of processed logs. Therefore it is very important to have at disposal relatively accurate data regarding these characteristics of bark for particular tree species. The main goal of this paper is to investigate the thickness of the bark and its share in the volume of roundwood of Norway spruce. Materials and Methods: The research was carried out in the area of the Canton 10 of the Federation of Bosnia and Herzegovina and it encompassed 393 trees of Norway spruce from 10 cm to 115 cm of thickness at breast height. Measuring of the mean diameter and double thickness of bark was conducted by section method. In total, 4,647 diameters and bark thicknesses were measured in different relative lengths of stems or in average 10.6 measurements per one stem. Results: As an optimal model for the evaluation of double thickness of the bark of Norway spruce depending on mean diameter of roundwood the function with designated determination coefficient of 0.7142 was selected. The obtained results have confirmed the previously defined relations of investigate characteristics, which are as following: a) with the increase of mean diameter of roundwood (section) double bark thickness is increased from 9.26 mm (thickness class 12.5 cm) to 31.65 mm (thickness class 92.5 cm); b) with the increase of mean diameter of roundwood the share of bark in its volume decreased from 14.26% (thickness class 12.5 cm) to 6.73% (thickness class 92.5 cm). Conclusions: By the actual method of estimating bark thickness or the share of bark in the volume of roundwood of Norway spruce in the forestry of the Federation of Bosnia and Herzegovina a significant error was created which increases with the increase of mean diameter.